Distribution characteristics and controlling factors of typical heavy metals in Huanghe River estuary, China
Lu Yuxi1; Pan Dawei2; Yang Tingting3; Wang Chenchen2
发表期刊JOURNAL OF OCEANOLOGY AND LIMNOLOGY
ISSN2096-5508
2023
卷号41期号:1页码:150-165
关键词colloidal heavy metal size fraction Huanghe (Yellow) River estuary geochemical feature
英文摘要The geochemical characteristics and potential controlling factors of colloidal Zn, Cd, and Pb in Huanghe (Yellow) River estuary (HRE), China were investigated. The three metals were highly variable over a range of spatiotemporal scales, comprehensively forced by various physical and biological processes. Total dissolved Zn, Cd, and Pb varied from 200.1 to 321.7, 2.6 to 4.1, and 0.5 to 1.0 nmol/L, respectively. Only one near-estuarine station of Zn had contamination factor values >1, which indicate the lower contaminant levels. Five dissolved species of Zn, Cd and Pb were fractionated, namely <1 kDa, 1-3 kDa, 3-10 kDa, 10-100 kDa, and 100 kDa-0.45 μm. The <1 kDa truly dissolved phase was the main fraction of the three dissolved metals (50%-62%), while the 100-kDa-0.45-μm high molecular weight colloidal fraction was dominant in their respective colloidal phase. Territorial input and sediment acted as important sources of strong ligands and natural colloids for the HRE water system. <3-kDa Zn and Pb were susceptible to the dissolved oxygen, the behaviors of colloidal Zn and 3-10-kDa Pb were related to dissolved organic carbon (DOC). However, no significant correlation between each dissolved fraction of Cd and salinity, pH, temperature, colloidal organic carbon, and DOC was found in this study. Overall, these findings, completed by the evaluation of the dissolved species of Zn, Cd, and Pb at 10 sites over the river-sea mixing zone, provided new insights into the colloidal heterogeneity that affect metals geochemical features, migration and fate in estuaries.
语种英语
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/36428
专题中国科学院海岸带环境过程与生态修复重点实验室
中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境工程技术研究与发展中心
作者单位1.中国科学院海洋研究所
2.中国科学院烟台海岸带研究所
3.烟台大学
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Lu Yuxi,Pan Dawei,Yang Tingting,et al. Distribution characteristics and controlling factors of typical heavy metals in Huanghe River estuary, China[J]. JOURNAL OF OCEANOLOGY AND LIMNOLOGY,2023,41(1):150-165.
APA Lu Yuxi,Pan Dawei,Yang Tingting,&Wang Chenchen.(2023).Distribution characteristics and controlling factors of typical heavy metals in Huanghe River estuary, China.JOURNAL OF OCEANOLOGY AND LIMNOLOGY,41(1),150-165.
MLA Lu Yuxi,et al."Distribution characteristics and controlling factors of typical heavy metals in Huanghe River estuary, China".JOURNAL OF OCEANOLOGY AND LIMNOLOGY 41.1(2023):150-165.
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