| Hydrophilic Multitemplate Molecularly Imprinted Biopolymers Based on a Green Synthesis Strategy for Determination of B-Family Vitamins | |
Ostovan, Abbas; Ghaedi, Mehrorang; Arabi, Maryam; Yang, Qian; Li, Jinhua ; Chen, Lingxin
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| 发表期刊 | ACS APPLIED MATERIALS & INTERFACES
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| ISSN | 1944-8244 |
| 2018-01-31 | |
| 卷号 | 10期号:4页码:4140-4150 |
| 关键词 | molecularly imprinted polymers multitemplate imprinting green synthesis dispersive solid-phase extraction experimental design vitamins |
| 研究领域 | Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
| DOI | 10.1021/acsami.7b17500 |
| 产权排序 | [Ostovan, Abbas] Islamic Azad Univ, Kerman Branch, Dept Chem, Kerman, Iran; [Ghaedi, Mehrorang; Arabi, Maryam] Univ Yasuj, Chem Dept, Yasuj 7591874831, Iran; [Yang, Qian; Li, Jinhua; Chen, Lingxin] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China |
| 作者部门 | 海岸带环境工程技术研究与发展中心 |
| 英文摘要 | A novel green synthesis strategy was proposed for preparation of multitemplate molecularly imprinted biopolymers (mt-MIBP) in aqueous media with less consumption of organic solvents, which were subsequently used as sorbents of ultrasound-assisted dispersive solid-phase extraction (d-SPE) for simultaneous recognition and efficient separation of B-family vitamins in juice samples, followed by high performance liquid chromatography (HPLC) determination. The obtained mt-MIBP was fully characterized by SEM, FT-IR, TEM, and BET. It offered high binding capacity, good selectivity, and fast dynamics toward all the templates. Involved parameters in the d-SPE efficiency such as mt-MIBP mass, sonication time, and eluting/washing solvents' types and volumes were concurrently investigated by central composite design with rapidity and reliability. Under the optimum conditions, the developed mt-MIBP-d-SPE-HPLC method exhibited wide linear range, low limits of detection and quantification (LOQs) within 1.2-5.5 mu g L-1 and 4.0-18.4 mu g L-1, respectively, and appropriate repeatability (relative standard deviation values below 4.2%, n = 4). The high selectivity of this method makes it suitable for successful monitoring of vitamins in juice samples with satisfactory recoveries of 75.8-92.7%, 81.1-92.5%, and 84.7-93.8% for vitamins riboflavin (B-2), nicotinamide (B-3), and pyridoxine (B-6), respectively. The present study implied highly promising perspectives of water-compatible eco-friendly mt-MIBP for highly effective multiresidue analysis in complicated matrixes. |
| 文章类型 | Article |
| 资助机构 | Graduate School of Yasouj University ; Research Council of Yasouj University ; National Natural Science Foundation of China [21477160, 41776110] ; National Defense Science and Technology Innovation Project of Chinese Academy of Sciences [CXJJ-16M254] |
| 收录类别 | SCI |
| 语种 | 英语 |
| 关键词[WOS] | WATER-SOLUBLE VITAMINS ; PERFORMANCE LIQUID-CHROMATOGRAPHY ; SOLID-PHASE EXTRACTION ; POROUS CARBON MICROSPHERES ; EXPERIMENTAL-DESIGN ; SELECTIVE REMOVAL ; MASS-SPECTROMETRY ; HYDROTHERMAL CARBONIZATION ; ACIDIC PHARMACEUTICALS ; SAMPLE PREPARATION |
| 研究领域[WOS] | Science & Technology - Other Topics ; Materials Science |
| WOS记录号 | WOS:000424728800111 |
| 引用统计 | |
| 文献类型 | 期刊论文 |
| 条目标识符 | http://ir.yic.ac.cn/handle/133337/24402 |
| 专题 | 中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境工程技术研究与发展中心 中国科学院海岸带环境过程与生态修复重点实验室 |
| 作者单位 | 1.Islamic Azad Univ, Kerman Branch, Dept Chem, Kerman, Iran; 2.Univ Yasuj, Chem Dept, Yasuj 7591874831, Iran; 3.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China |
| 推荐引用方式 GB/T 7714 | Ostovan, Abbas,Ghaedi, Mehrorang,Arabi, Maryam,et al. Hydrophilic Multitemplate Molecularly Imprinted Biopolymers Based on a Green Synthesis Strategy for Determination of B-Family Vitamins[J]. ACS APPLIED MATERIALS & INTERFACES,2018,10(4):4140-4150. |
| APA | Ostovan, Abbas,Ghaedi, Mehrorang,Arabi, Maryam,Yang, Qian,Li, Jinhua,&Chen, Lingxin.(2018).Hydrophilic Multitemplate Molecularly Imprinted Biopolymers Based on a Green Synthesis Strategy for Determination of B-Family Vitamins.ACS APPLIED MATERIALS & INTERFACES,10(4),4140-4150. |
| MLA | Ostovan, Abbas,et al."Hydrophilic Multitemplate Molecularly Imprinted Biopolymers Based on a Green Synthesis Strategy for Determination of B-Family Vitamins".ACS APPLIED MATERIALS & INTERFACES 10.4(2018):4140-4150. |
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