Characteristics of dissolved organic matter (DOM) and relationship with dissolved mercury in Xiaoqing River-Laizhou Bay estuary, Bohai Sea, China
Jiang, Tao1,2; Skyllberg, Ulf2; Bjorn, Erik4; Green, Nelson W.5; Tang, Jianhui3; Wang, Dingyong1; Gao, Jie1; Li, Chuxian1; Wang, DY (reprint author), Southwest Univ, Key Lab Ecoenvironm Gorges Reservoir Reg 3, Chongqing Key Lab Agr Resources & Environm, Minist Educ,Coll Resources & Environm,Dept Enviro, Chongqing 400716, Peoples R China.
发表期刊ENVIRONMENTAL POLLUTION
ISSN0269-7491
2017-04-01
卷号223页码:19-30
关键词Dissolved Organic Matter Fluorescence Uv-vis Absorption Bohai Sea Laizhou Bay Mercury
DOI10.1016/j.envpol.2016.12.006
产权排序[Jiang, Tao; Wang, Dingyong; Gao, Jie; Li, Chuxian] Southwest Univ, Key Lab Ecoenvironm Gorges Reservoir Reg 3, Chongqing Key Lab Agr Resources & Environm, Minist Educ,Coll Resources & Environm,Dept Enviro, Chongqing 400716, Peoples R China; [Jiang, Tao; Skyllberg, Ulf] Swedish Univ Agr Sci, Dept Forest Ecol & Management, SE-90183 Umea, Sweden; [Tang, Jianhui] Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China; [Bjorn, Erik] Umea Univ, Dept Chem, SE-90187 Umea, Sweden; [Green, Nelson W.] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA
作者部门中科院海岸带环境过程与生态修复重点实验室
英文摘要Because of heterogeneous properties, dissolved organic matter (DOM) is known to control the environmental fate of a variety of organic pollutants and trace metals in aquatic systems. Here we report absorptive and fluorescence properties of DOM, in concurrence with concentrations of dissolved mercury (Hg), along the Xiaoqing River-Laizhou Bay estuary system located in the Bohai Sea of China. A mixing model consisting of the two end-members terrestrial and aquatic DOM demonstrated that terrestrial signatures decreased significantly from the river into the estuary. Quasi-conservative mixing behavior of DOM sources suggests that the variations in the average DOM composition were governed by physical processes (e.g., dilution) rather than by new production and/or degradation processes. In contrast to some previous studies of river-estuary systems, the Xiaoqing River-Laizhou Bay estuary system displayed a non-significant correlation between DOM and Hg quantities. Based on this and the variation of Hg concentration along the salinity gradient, we concluded that Hg showed a non-conservative mixing behavior of suggested end-member sources. Thus, rather than mixing, Hg concentration variations seemed to be controlled by biogeochemical processes. (C) 2016 Elsevier Ltd. All rights reserved.
文章类型Article
资助机构National Science Foundation of China(41403079) ; National Key Basic Research Program of China (973 Program)(2013CB430004) ; Key Research Programs of the Chinese Academy of Sciences(KZZD-EW-14 ; Swedish Research Council (VR)(621-2014-5370) ; XDA11020402)
收录类别SCI
语种英语
关键词[WOS]MIDDLE ATLANTIC BIGHT ; BALTIC SEA ; FLUORESCENCE SPECTROSCOPY ; CHESAPEAKE BAY ; NONCONSERVATIVE BEHAVIOR ; ULTRAVIOLET ABSORBENCY ; AQUATIC ENVIRONMENT ; HUMIC SUBSTANCES ; YANGTZE ESTUARY ; TRACE-METALS
研究领域[WOS]Environmental Sciences & Ecology
WOS记录号WOS:000397359500003
引用统计
被引频次:95[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/22060
专题中国科学院海岸带环境过程与生态修复重点实验室
通讯作者Wang, DY (reprint author), Southwest Univ, Key Lab Ecoenvironm Gorges Reservoir Reg 3, Chongqing Key Lab Agr Resources & Environm, Minist Educ,Coll Resources & Environm,Dept Enviro, Chongqing 400716, Peoples R China.
作者单位1.Southwest Univ, Key Lab Ecoenvironm Gorges Reservoir Reg 3, Chongqing Key Lab Agr Resources & Environm, Minist Educ,Coll Resources & Environm,Dept Enviro, Chongqing 400716, Peoples R China
2.Swedish Univ Agr Sci, Dept Forest Ecol & Management, SE-90183 Umea, Sweden
3.Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China
4.Umea Univ, Dept Chem, SE-90187 Umea, Sweden
5.Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA
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GB/T 7714
Jiang, Tao,Skyllberg, Ulf,Bjorn, Erik,et al. Characteristics of dissolved organic matter (DOM) and relationship with dissolved mercury in Xiaoqing River-Laizhou Bay estuary, Bohai Sea, China[J]. ENVIRONMENTAL POLLUTION,2017,223:19-30.
APA Jiang, Tao.,Skyllberg, Ulf.,Bjorn, Erik.,Green, Nelson W..,Tang, Jianhui.,...&Wang, DY .(2017).Characteristics of dissolved organic matter (DOM) and relationship with dissolved mercury in Xiaoqing River-Laizhou Bay estuary, Bohai Sea, China.ENVIRONMENTAL POLLUTION,223,19-30.
MLA Jiang, Tao,et al."Characteristics of dissolved organic matter (DOM) and relationship with dissolved mercury in Xiaoqing River-Laizhou Bay estuary, Bohai Sea, China".ENVIRONMENTAL POLLUTION 223(2017):19-30.
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