Distribution and long-range transport of polyfluoroalkyl substances in the Arctic, Atlantic Ocean and Antarctic coast
Zhao, Zhen1,2,3; Xie, Zhiyong1; Moeller, Axel1; Sturm, Renate1; Tang, Jianhui2; Zhang, Gan4; Ebinghaus, Ralf1
发表期刊ENVIRONMENTAL POLLUTION
ISSN0269-7491
2012-11-01
卷号170页码:71-77
关键词Polyfluoroalkyl Substances (Pfass) Seawater Marine Environment Long-range Transport
产权排序[Zhao, Zhen; Xie, Zhiyong; Moeller, Axel; Sturm, Renate; Ebinghaus, Ralf] Helmotz Zentrum Geesthacht, Ctr Mat & Coastal Res, Inst Coastal Res, Geesthacht, Germany; [Zhao, Zhen; Tang, Jianhui] Chinese Acad Sci, Key Lab Coastal Zone Environm Proc, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China; [Zhao, Zhen] Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China; [Zhang, Gan] Chinese Acad Sci, Guangzhou Geochem Inst, Guangzhou 590640, Guangdong, Peoples R China
通讯作者Xie, ZY (reprint author), Helmotz Zentrum Geesthacht, Ctr Mat & Coastal Res, Inst Coastal Res, Geesthacht, Germany.
作者部门中科院海岸带环境过程与生态修复重点实验室
英文摘要The global distribution and long-range transport of polyfluoroalkyl substances (PFASs) were investigated using seawater samples collected from the Greenland Sea, East Atlantic Ocean and the Southern Ocean in 2009-2010. Elevated levels of Sigma PFASs were detected in the North Atlantic Ocean with the concentrations ranging from 130 to 650 pg/L In the Greenland Sea, the Sigma PFASs concentrations ranged from 45 to 280 pg/L, and five most frequently detected compounds were perfluorooctanoic acid (PFOA), perfluorohexanesulfonate (PFHxS), perfluorohexanoic acid (PFHxA), perfluorooctane sulfonate (PFOS) and perfluorobutane sulfonate (PFBS). PFOA (15 pg/L) and PFOS (25-45 pg/L) were occasionally found in the Southern Ocean. In the Atlantic Ocean, the Sigma PFASs concentration decreased from 2007 to 2010. The elevated PFOA level that resulted from melting snow and ice in Greenland Sea implies that the Arctic may have been driven by climate change and turned to be a source of PFASs for the marine ecosystem. (c) 2012 Elsevier Ltd. All rights reserved.; The global distribution and long-range transport of polyfluoroalkyl substances (PFASs) were investigated using seawater samples collected from the Greenland Sea, East Atlantic Ocean and the Southern Ocean in 2009-2010. Elevated levels of Sigma PFASs were detected in the North Atlantic Ocean with the concentrations ranging from 130 to 650 pg/L In the Greenland Sea, the Sigma PFASs concentrations ranged from 45 to 280 pg/L, and five most frequently detected compounds were perfluorooctanoic acid (PFOA), perfluorohexanesulfonate (PFHxS), perfluorohexanoic acid (PFHxA), perfluorooctane sulfonate (PFOS) and perfluorobutane sulfonate (PFBS). PFOA (15 pg/L) and PFOS (25-45 pg/L) were occasionally found in the Southern Ocean. In the Atlantic Ocean, the Sigma PFASs concentration decreased from 2007 to 2010. The elevated PFOA level that resulted from melting snow and ice in Greenland Sea implies that the Arctic may have been driven by climate change and turned to be a source of PFASs for the marine ecosystem. (c) 2012 Elsevier Ltd. All rights reserved.
文章类型Article
收录类别SCI
语种英语
关键词[WOS]PERSISTENT ORGANIC POLLUTANTS ; PERFLUORINATED COMPOUNDS ; ATMOSPHERIC CHEMISTRY ; GLOBAL DISTRIBUTION ; CLIMATE-CHANGE ; SURFACE-WATER ; SEA-ICE ; ACIDS ; RIVER ; FATE
研究领域[WOS]Environmental Sciences & Ecology
WOS记录号WOS:000308450100010
引用统计
被引频次:123[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/5978
专题中国科学院海岸带环境过程与生态修复重点实验室
作者单位1.Helmotz Zentrum Geesthacht, Ctr Mat & Coastal Res, Inst Coastal Res, Geesthacht, Germany
2.Chinese Acad Sci, Key Lab Coastal Zone Environm Proc, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China
3.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
4.Chinese Acad Sci, Guangzhou Geochem Inst, Guangzhou 590640, Guangdong, Peoples R China
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GB/T 7714
Zhao, Zhen,Xie, Zhiyong,Moeller, Axel,et al. Distribution and long-range transport of polyfluoroalkyl substances in the Arctic, Atlantic Ocean and Antarctic coast[J]. ENVIRONMENTAL POLLUTION,2012,170:71-77.
APA Zhao, Zhen.,Xie, Zhiyong.,Moeller, Axel.,Sturm, Renate.,Tang, Jianhui.,...&Ebinghaus, Ralf.(2012).Distribution and long-range transport of polyfluoroalkyl substances in the Arctic, Atlantic Ocean and Antarctic coast.ENVIRONMENTAL POLLUTION,170,71-77.
MLA Zhao, Zhen,et al."Distribution and long-range transport of polyfluoroalkyl substances in the Arctic, Atlantic Ocean and Antarctic coast".ENVIRONMENTAL POLLUTION 170(2012):71-77.
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