Institutional Repository of Key Laboratory of Coastal Zone Environmental Processes, Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences (KLCEP)
Source Apportionment and Toxic Potency of PM2.5-Bound Polycyclic Aromatic Hydrocarbons (PAHs) at an Island in the Middle of Bohai Sea, China | |
Qu, Lin1; Yang, Lin1; Zhang, Yinghong2; Wang, Xiaoping3,4,5; Sun, Rong4,5; Li, Bo6; Lv, Xiaoxue6; Chen, Yuehong1; Wang, Qin1; Tian, Chongguo4,5; Ji, Ling1 | |
发表期刊 | ATMOSPHERE |
2022-05-01 | |
卷号 | 13期号:5页码:15 |
关键词 | polycyclic aromatic hydrocarbons PM2.5 source apportionment toxic potency Bohai Sea |
DOI | 10.3390/atmos13050699 |
通讯作者 | Yang, Lin([email protected]) |
英文摘要 | Polycyclic aromatic hydrocarbons (PAHs) have attracted more attention because of their high atmospheric concentration and toxicity in recent decades. In this study, a total of 60 PM2.5 samples were collected from Beihuangcheng Island in Bohai Sea, China, from August 2017 to March 2018 for analyzing 16 congeners of PAHs (Sigma(16)PAHs). Sources of PAHs were apportioned by a positive matrix factorization (PMF) model and the carcinogenic risk due to exposure to the PAHs was estimated by the toxicity equivalent of BaP (BaPeq). The results showed that the average concentration of Sigma(16)PAHs was 35.3 +/- 41.8 ng/m(3). The maximum concentration of Sigma(16)PAHs occurred in winter, followed by spring and autumn, and summer. The PMF modeling apportioned the PAHs into four sources, coal combustion, biomass burning, vehicle exhaust, and petroleum release, contributing 43.1%, 25.8%, 24.7%, and 6.39%, respectively. The average Sigma BaPeq concentration was 2.32 +/- 4.95 ng/m(3) during the sampling period, and vehicle exhaust was the largest contributor. The finding indicates that more attention should be paid to reduce the emissions from coal combustion and vehicle exhaust because they were the largest contributors to the PAH concentration in PM2.5 and Sigma BaPeq concentration, respectively. |
资助机构 | Marine Science and Technology Project of Beihai Branch, Ministry of Natural Resources of China ; National Natural Science Foundation of China ; seed project of Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences |
收录类别 | SCI |
语种 | 英语 |
关键词[WOS] | REGIONAL BACKGROUND SITE ; DIAGNOSTIC RATIOS ; ATMOSPHERIC LEVELS ; HEALTH-RISK ; PM2.5 ; EMISSION ; PATTERNS ; INVENTORY ; GUANGZHOU ; EXPOSURE |
研究领域[WOS] | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
WOS记录号 | WOS:000803456100001 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.yic.ac.cn/handle/133337/37528 |
专题 | 中国科学院海岸带环境过程与生态修复重点实验室 中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室 |
通讯作者 | Yang, Lin |
作者单位 | 1.State Ocean Adm SOA, Yantai Ocean Environm Monitoring Cent Stn, Yantai 264006, Peoples R China 2.Yantai Ecol Environm Monitoring Ctr Shandong Prov, Yantai 264000, Peoples R China 3.Ludong Univ, Sch Resources & Environm Engn, Yantai 264025, Peoples R China 4.Chinese Acad Sci, Yantai Inst Coastal Zone Res, CAS Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China 5.Shandong Key Lab Coastal Environm Proc, Yantai 264003, Peoples R China 6.Yantai Environm Monitoring Ctr, Yantai 264003, Peoples R China |
推荐引用方式 GB/T 7714 | Qu, Lin,Yang, Lin,Zhang, Yinghong,et al. Source Apportionment and Toxic Potency of PM2.5-Bound Polycyclic Aromatic Hydrocarbons (PAHs) at an Island in the Middle of Bohai Sea, China[J]. ATMOSPHERE,2022,13(5):15. |
APA | Qu, Lin.,Yang, Lin.,Zhang, Yinghong.,Wang, Xiaoping.,Sun, Rong.,...&Ji, Ling.(2022).Source Apportionment and Toxic Potency of PM2.5-Bound Polycyclic Aromatic Hydrocarbons (PAHs) at an Island in the Middle of Bohai Sea, China.ATMOSPHERE,13(5),15. |
MLA | Qu, Lin,et al."Source Apportionment and Toxic Potency of PM2.5-Bound Polycyclic Aromatic Hydrocarbons (PAHs) at an Island in the Middle of Bohai Sea, China".ATMOSPHERE 13.5(2022):15. |
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