Metal-Organic Framework-Based Composites for the Adsorption Removal of Per- and Polyfluoroalkyl Substances from Water

doi:10.1021/acs.langmuir.3c02939

YIC-IR

	Metal-Organic Framework-Based Composites for the Adsorption Removal of Per- and Polyfluoroalkyl Substances from Water
	Li, Shuang 1; Ma, Jiping 1; Cheng, Jiawen 1; Wu, Gege 1; Wang, Shasha 1; Huang, Chaonan 1; Li, Jinhua2,3 ; Chen, Lingxin2,3,4
发表期刊	LANGMUIR
ISSN	0743-7463
	2024-02-01
卷号	40 期号:6 页码:2815-2829
DOI	10.1021/acs.langmuir.3c02939
通讯作者	Ma, Jiping([email protected]) ; Chen, Lingxin([email protected])
英文摘要	The increasing health risks posed by per- and polyfluoroalkyl substances (PFASs) in the environment highlight the importance of implementing effective removal techniques. Conventional wastewater treatment processes are inadequate for removing persistent organic pollutants. Recent studies have increasingly demonstrated that metal-organic frameworks (MOFs) are capable of removing PFASs from water through adsorption techniques. However, there is still constructive discussion on the potential of MOFs in adsorbing and removing PFASs for large-scale engineering applications. This review systematically investigates the use of MOFs as adsorbents for the removal of PFAS in water treatment. This primarily involved a comprehensive analysis of existing literature to understand the adsorption mechanisms of MOFs and to identify factors that enhance their efficiency in removing PFASs. We also explore the critical aspects of regeneration and stability of MOFs, assessing their reusability and long-term performance, which are essential for large-scale water treatment applications. Finally, our study highlights the challenges of removing PFASs using MOFs. Especially, the efficient removal of short-chain PFASs with hydrophilicity is a major challenge, while medium- to long-chain PFASs are frequently susceptible to being captured from water by MOFs through multiple synergistic effects. The ion-exchange force may be the key to solving this difficulty, but its susceptibility to ion interference in water needs to be addressed in practical applications. We hope that this review can provide valuable insights into the effective removal and adsorption mechanisms of PFASs as well as advance the sustainable utilization of MOFs in the field of water treatment, thereby presenting a novel perspective.
资助机构	National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Natural Science Foundation of Shandong Province of China ; Taishan Scholar Project Special Funding
收录类别	SCI
语种	英语
关键词[WOS]	PERFLUOROOCTANE SULFONATE ; PERFLUORINATED COMPOUNDS ; PERFLUOROALKYL ACIDS ; EFFICIENT REMOVAL ; HIGH-PERFORMANCE ; SORPTION ; PFOA ; MOFS ; ADSORBENT ; MECHANISM
研究领域[WOS]	Chemistry ; Materials Science
WOS记录号	WOS:001159207300001
引用统计	被引频次：5[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.yic.ac.cn/handle/133337/34868
专题	中国科学院烟台海岸带研究所
通讯作者	Ma, Jiping; Chen, Lingxin
作者单位	1.Qingdao Univ Technol, Sch Environm & Municipal Engn, Qingdao 266033, Shandong, Peoples R China 2.Chinese Acad Sci, Yantai Inst Coastal Zone Res, CAS Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Shandong, Peoples R China 3.Shaoxing Univ, Coll Chem & Chem Engn, Shaoxing 312000, Zhejiang, Peoples R China 4.Binzhou Med Univ, Sch Pharm, Yantai 264003, Shandong, Peoples R China
推荐引用方式 GB/T 7714	Li, Shuang,Ma, Jiping,Cheng, Jiawen,et al. Metal-Organic Framework-Based Composites for the Adsorption Removal of Per- and Polyfluoroalkyl Substances from Water[J]. LANGMUIR,2024,40(6):2815-2829.
APA	Li, Shuang.,Ma, Jiping.,Cheng, Jiawen.,Wu, Gege.,Wang, Shasha.,...&Chen, Lingxin.(2024).Metal-Organic Framework-Based Composites for the Adsorption Removal of Per- and Polyfluoroalkyl Substances from Water.LANGMUIR,40(6),2815-2829.
MLA	Li, Shuang,et al."Metal-Organic Framework-Based Composites for the Adsorption Removal of Per- and Polyfluoroalkyl Substances from Water".LANGMUIR 40.6(2024):2815-2829.