YIC-IR
Dual-isotope-based source apportionment of nitrate in 30 rivers draining into the Bohai Sea, north China
Yu, Jing1,7; Zhang, Wei2; Tan, Yang1,7; Zong, Zheng1,7; Hao, Qinqin3; Tian, Chongguo1,7; Zhang, Hua1; Li, Jun4,5; Fang, Yunting6; Zhang, Gan4,5
发表期刊ENVIRONMENTAL POLLUTION
ISSN0269-7491
2021-08-15
卷号283页码:8
关键词Dual-isotope Fluvial nitrate Source apportionment Flux Bayesian Bohai sea
DOI10.1016/j.envpol.2021.117112
通讯作者Zong, Zheng([email protected])
英文摘要Excessive nitrate (NO3-) in rivers can lead to water quality deterioration, and can also be directly input into estuaries and oceans, thus posing a serious threat to the stability of their ecosystems. In this study, the concentration, isotopes and sources of NO3- in 30 rivers discharging into the Bohai Sea were comprehensively investigated. The mean concentration of NO3--N was 2.24 +/- 2.11 mg L-1, with obvious seasonal and spatial variations. In total, 104.24 kt of NO3--N was discharged into the Bohai Sea annually, to which the Yellow River Basin and Liao River Basin made the largest contributions. The range of delta N-15-NO3- was -1.1 parts per thousand to +33.2 parts per thousand (mean value, +11.4 +/- 5.0 parts per thousand), with no significant seasonal or spatial differences; the mean value of delta O-18-NO3- was +9.4 +/- 7.2 parts per thousand, with much higher values seen in June. Based on the MixSIAR model, manure (24.3 +/- 7.5%) and sewage (19.1 +/- 14.5%) were the primary sources of NO3- in the 30 rivers, followed by NO3- fertilizers (16.3 +/- 12.5%), soil N (15.5 +/- 11.9%), atmospheric deposition of NO3- (13.5 +/- 5.7%) and NH4+ fertilizers (11.4 +/- 8.9%). This finding highlights the vital roles of sewage and manure management in riverine NO3-. Using a mathematical method, the contributions of various sources to each river were simulated. The results indicated that management of the Yellow River, Daliao River, Liao River, and Xiaoqing River is more urgently needed than that of other rivers to control Bohai NO3- pollution. We believe that this finding will provide guidance for scientific management of NO3- pollution in these 30 rivers and the Bohai Sea. (C) 2021 Elsevier Ltd. All rights reserved.
资助机构Natural Scientific Foundation of China (NSFC) ; NSFC-Shandong Joint Fund
收录类别SCI
语种英语
关键词[WOS]REGIONAL BACKGROUND SITE ; MIXING MODEL ; YELLOW-RIVER ; FRESH-WATER ; NOX SOURCES ; NITROGEN ; DISCHARGE ; QUANTIFICATION ; NITRIFICATION ; POLLUTION
研究领域[WOS]Environmental Sciences & Ecology
WOS记录号WOS:000663133200012
引用统计
被引频次:23[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/34775
专题中国科学院烟台海岸带研究所
通讯作者Zong, Zheng
作者单位1.Chinese Acad Sci, CAS Key Lab Coastal Environm Proc & Ecol Remediat, Shandong Key Lab Coastal Environm Proc, Yantai Inst Coastal Zone Res YIC,YICCAS, Yantai 264003, Shandong, Peoples R China
2.Yantai Univ, Sch Environm & Mat Engn, Yantai 264005, Shandong, Peoples R China
3.Guangdong Acad Sci, Natl Reg Joint Engn Res Ctr Soil Pollut Control &, Guangdong Key Lab Integrated Agroenvironm Pollut, Inst Ecoenvironm & Soil Sci, Guangzhou 510650, Peoples R China
4.Chinese Acad Sci, State Key Lab Organ Geochem, Guangzhou Inst Geochem, Guangzhou 510640, Peoples R China
5.Chinese Acad Sci, Guangdong Key Lab Environm Protect & Resources Ut, Guangzhou Inst Geochem, Guangzhou 510640, Peoples R China
6.Chinese Acad Sci, Inst Appl Ecol, CAS Key Lab Forest Ecol & Management, Shenyang 110164, Liaoning, Peoples R China
7.Chinese Acad Sci, Ctr Ocean Megasci, Qingdao 266071, Peoples R China
推荐引用方式
GB/T 7714
Yu, Jing,Zhang, Wei,Tan, Yang,et al. Dual-isotope-based source apportionment of nitrate in 30 rivers draining into the Bohai Sea, north China[J]. ENVIRONMENTAL POLLUTION,2021,283:8.
APA Yu, Jing.,Zhang, Wei.,Tan, Yang.,Zong, Zheng.,Hao, Qinqin.,...&Zhang, Gan.(2021).Dual-isotope-based source apportionment of nitrate in 30 rivers draining into the Bohai Sea, north China.ENVIRONMENTAL POLLUTION,283,8.
MLA Yu, Jing,et al."Dual-isotope-based source apportionment of nitrate in 30 rivers draining into the Bohai Sea, north China".ENVIRONMENTAL POLLUTION 283(2021):8.
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