The first high resolution PAH record of industrialization over the past 200 years in Liaodong Bay, northeastern China | |
Guo, Fei1,2; Gao, Maosheng3; Dong, Junfu1; Sun, Jun3; Hou, Guohua3; Liu, Sen5; Du, Xiaojing4; Yang, Shu1; Liu, Jihua1,6; Huang, Yongsong4 | |
发表期刊 | WATER RESEARCH |
ISSN | 0043-1354 |
2022-10-01 | |
卷号 | 224页码:11 |
关键词 | PAHs Fire history Industrial revolution Diagnostic ratios Anthropogenic CO2 emission |
DOI | 10.1016/j.watres.2022.119103 |
通讯作者 | Guo, Fei([email protected]) ; Liu, Jihua([email protected]) ; Huang, Yongsong([email protected]) |
英文摘要 | Polycyclic aromatic hydrocarbons (PAHs) are excellent tracers for fossil fuel combustion, natural fires and petroleum contamination, and have been widely used for reconstructing past wildfires and industrial activities at a variety of time scales. Here, for the first time, we obtain a high resolution (annual to decadal scale) record of PAHs from two parallel marine sediment cores from the Liaodong Bay, Northeastern China to reconstruct the industrial activities, spanning the past similar to 200 years from 1815 to 2014. Our data indicate that PAH variations can be divided into four episodes: I) low (probably near background) PAHs from natural fires and domestic wood combustion during the pre-industrial period from 1815 to 1890; II) slightly increased (but with large fluctuations) PAH concentrations derived from intermittent warfare during the World War (1891-1945) and increased industrial activities after 1946 (1946-1965); III) a period of stagnation and, in some cases, reduction in PAHs during the "Cultural Revolution" (1966 to 1979); and IV) a rapid and persistent rise in PAHs post 1979 linked to fast economic development, with PAH concentrations doubled from 1979 to 2014. Changes in PAH distributions demonstrate major shifts in the dominant types of fuels over time from vegetation/wood, to coal and wood, followed by coal and petroleum (including vehicle emissions) over the past 200 years. We find that PAH records also show similar trend to domestic economy and the estimated regional Anthropocene CO2 emissions from industrial activities, suggesting sedimentary PAH fluxes could be used as an indirect and qualitative proxy to track the trend for regional anthropogenic CO2 emissions. |
资助机构 | National Natural Science Foundation of China ; Science Foundation for Young Scientists of Shandong Province ; Chinese Geological Survey program |
收录类别 | SCI |
语种 | 英语 |
关键词[WOS] | POLYCYCLIC AROMATIC-HYDROCARBONS ; PEARL RIVER ESTUARY ; CONTINENTAL-SHELF ; SEDIMENT CORE ; YELLOW-RIVER ; SOURCE IDENTIFICATION ; DIAGNOSTIC RATIOS ; TEMPORAL TRENDS ; LAKE-SEDIMENTS ; CONTAMINATION |
研究领域[WOS] | Engineering ; Environmental Sciences & Ecology ; Water Resources |
WOS记录号 | WOS:000861750600001 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.yic.ac.cn/handle/133337/31758 |
专题 | 中国科学院烟台海岸带研究所 |
通讯作者 | Guo, Fei; Liu, Jihua; Huang, Yongsong |
作者单位 | 1.Shandong Univ Qingdao, Inst Marine Sci & Technol, Qingdao 266237, Peoples R China 2.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Peoples R China 3.China Geol Survey, Qingdao Inst Marine Geol, Qingdao 266071, Peoples R China 4.Brown Univ, Dept Earth Environm & Planetary Sci, Providence, RI 02912 USA 5.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China 6.Southern Marine Sci & Engn Guangdong Lab Zhuhai, Guangzhou 510000, Peoples R China |
推荐引用方式 GB/T 7714 | Guo, Fei,Gao, Maosheng,Dong, Junfu,et al. The first high resolution PAH record of industrialization over the past 200 years in Liaodong Bay, northeastern China[J]. WATER RESEARCH,2022,224:11. |
APA | Guo, Fei.,Gao, Maosheng.,Dong, Junfu.,Sun, Jun.,Hou, Guohua.,...&Huang, Yongsong.(2022).The first high resolution PAH record of industrialization over the past 200 years in Liaodong Bay, northeastern China.WATER RESEARCH,224,11. |
MLA | Guo, Fei,et al."The first high resolution PAH record of industrialization over the past 200 years in Liaodong Bay, northeastern China".WATER RESEARCH 224(2022):11. |
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