Fates and ecological effects of current-use pesticides (CUPs) in a typical river-estuarine system of Laizhou Bay, North China
Zhen, XM; Liu, L; Wang, XM; Zhong, GC; Tang, JH
发表期刊ENVIRONMENTAL POLLUTION
ISSN0269-7491
2019-09
卷号252期号:A页码:573-579
关键词Current-use pesticides River-estuary Fates Distribution Chlorpyrifos
研究领域Environmental Sciences
DOI10.1016/j.envpol.2019.05.141
产权排序[Zhen, Xiaomei; Liu, Lin; Wang, Xinming; Zhong, Guangcai] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Beijing 510631, Peoples R China; [Zhen, Xiaomei; Liu, Lin; Tang, Jianhui] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China; [Zhen, Xiaomei; Liu, Lin] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
通讯作者Tang, Jianhui([email protected])
作者部门海岸带环境过程实验室
英文摘要Current-use pesticides (CUPS) are widely applied in agriculture; however, little is known about their environmental behaviors, especially in the freshwater-seawater transitional zone. Water and sediment samples were collected in an intensively human impacted river (Xiaoqing River) from the headwaters to Laizhou Bay to investigate the distributions and environmental fates of four CUPs: trifluralin, chlorothalonil, chlorpyrifos, and dicofol. These CUPS were frequently detected in water and sediment samples. Sigma CUPs in water and sediment samples ranged from 1.20 to 100.2 ng L-1 and 6.6-2972.5 ng g(-1) dry weight (dw), respectively. Chlorpyrifos and chlorothalonil were the most abundant CUPs in water and sediment samples, respectively. Spatial distribution of CUPs in the Xiaoqing River aquatic ecosystem was mainly influenced by point sources, agricultural activities, the dilution effect by seawater, and environmental parameters. Field-based sediment water partitioning coefficients, normalized by organic carbon (log Koc), were calculated. Interestingly, temperature and salinity exhibited significant impacts on the distribution of log Koc of the four CUPs. The effect of temperature on the distribution of log Koc of the four CUPs varied between the CUPs. In most water samples, the levels of chlorpyrifos exceed the freshwater screening benchmarks. Hence, urgent control measures need to be devised and implemented. (C) 2019 Elsevier Ltd. All rights reserved.
文章类型Article
资助机构National Science Foundation of ChinaNational Natural Science Foundation of China [41773138, U1806207, 41503111] ; Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences [YIC Y855011024]
收录类别SCI
语种英语
关键词[WOS]POLYCYCLIC AROMATIC-HYDROCARBONS ; POLYBROMINATED DIPHENYL ETHERS ; FLAME RETARDANTS ; BOHAI SEA ; ORGANOCHLORINE PESTICIDES ; SPATIAL-DISTRIBUTION ; SEASONAL-VARIATION ; AIR ; SEDIMENTS ; SEAWATER
研究领域[WOS]Environmental Sciences
WOS记录号WOS:000483005500060
引用统计
被引频次:31[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/24874
专题中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室
中国科学院海岸带环境过程与生态修复重点实验室
作者单位1.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Beijing 510631, Peoples R China;
2.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China;
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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GB/T 7714
Zhen, XM,Liu, L,Wang, XM,et al. Fates and ecological effects of current-use pesticides (CUPs) in a typical river-estuarine system of Laizhou Bay, North China[J]. ENVIRONMENTAL POLLUTION,2019,252(A):573-579.
APA Zhen, XM,Liu, L,Wang, XM,Zhong, GC,&Tang, JH.(2019).Fates and ecological effects of current-use pesticides (CUPs) in a typical river-estuarine system of Laizhou Bay, North China.ENVIRONMENTAL POLLUTION,252(A),573-579.
MLA Zhen, XM,et al."Fates and ecological effects of current-use pesticides (CUPs) in a typical river-estuarine system of Laizhou Bay, North China".ENVIRONMENTAL POLLUTION 252.A(2019):573-579.
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