Fates and ecological effects of current-use pesticides (CUPs) in a typical river-estuarine system of Laizhou Bay, North China | |
Zhen, XM; Liu, L; Wang, XM; Zhong, GC; Tang, JH | |
发表期刊 | ENVIRONMENTAL POLLUTION |
ISSN | 0269-7491 |
2019-09 | |
卷号 | 252期号:A页码:573-579 |
关键词 | Current-use pesticides River-estuary Fates Distribution Chlorpyrifos |
研究领域 | Environmental Sciences |
DOI | 10.1016/j.envpol.2019.05.141 |
产权排序 | [Zhen, Xiaomei; Liu, Lin; Wang, Xinming; Zhong, Guangcai] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Beijing 510631, Peoples R China; [Zhen, Xiaomei; Liu, Lin; Tang, Jianhui] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China; [Zhen, Xiaomei; Liu, Lin] Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
通讯作者 | Tang, Jianhui([email protected]) |
作者部门 | 海岸带环境过程实验室 |
英文摘要 | Current-use pesticides (CUPS) are widely applied in agriculture; however, little is known about their environmental behaviors, especially in the freshwater-seawater transitional zone. Water and sediment samples were collected in an intensively human impacted river (Xiaoqing River) from the headwaters to Laizhou Bay to investigate the distributions and environmental fates of four CUPs: trifluralin, chlorothalonil, chlorpyrifos, and dicofol. These CUPS were frequently detected in water and sediment samples. Sigma CUPs in water and sediment samples ranged from 1.20 to 100.2 ng L-1 and 6.6-2972.5 ng g(-1) dry weight (dw), respectively. Chlorpyrifos and chlorothalonil were the most abundant CUPs in water and sediment samples, respectively. Spatial distribution of CUPs in the Xiaoqing River aquatic ecosystem was mainly influenced by point sources, agricultural activities, the dilution effect by seawater, and environmental parameters. Field-based sediment water partitioning coefficients, normalized by organic carbon (log Koc), were calculated. Interestingly, temperature and salinity exhibited significant impacts on the distribution of log Koc of the four CUPs. The effect of temperature on the distribution of log Koc of the four CUPs varied between the CUPs. In most water samples, the levels of chlorpyrifos exceed the freshwater screening benchmarks. Hence, urgent control measures need to be devised and implemented. (C) 2019 Elsevier Ltd. All rights reserved. |
文章类型 | Article |
资助机构 | National Science Foundation of ChinaNational Natural Science Foundation of China [41773138, U1806207, 41503111] ; Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences [YIC Y855011024] |
收录类别 | SCI |
语种 | 英语 |
关键词[WOS] | POLYCYCLIC AROMATIC-HYDROCARBONS ; POLYBROMINATED DIPHENYL ETHERS ; FLAME RETARDANTS ; BOHAI SEA ; ORGANOCHLORINE PESTICIDES ; SPATIAL-DISTRIBUTION ; SEASONAL-VARIATION ; AIR ; SEDIMENTS ; SEAWATER |
研究领域[WOS] | Environmental Sciences |
WOS记录号 | WOS:000483005500060 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.yic.ac.cn/handle/133337/24874 |
专题 | 中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室 中国科学院海岸带环境过程与生态修复重点实验室 |
作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Beijing 510631, Peoples R China; 2.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China; 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Zhen, XM,Liu, L,Wang, XM,et al. Fates and ecological effects of current-use pesticides (CUPs) in a typical river-estuarine system of Laizhou Bay, North China[J]. ENVIRONMENTAL POLLUTION,2019,252(A):573-579. |
APA | Zhen, XM,Liu, L,Wang, XM,Zhong, GC,&Tang, JH.(2019).Fates and ecological effects of current-use pesticides (CUPs) in a typical river-estuarine system of Laizhou Bay, North China.ENVIRONMENTAL POLLUTION,252(A),573-579. |
MLA | Zhen, XM,et al."Fates and ecological effects of current-use pesticides (CUPs) in a typical river-estuarine system of Laizhou Bay, North China".ENVIRONMENTAL POLLUTION 252.A(2019):573-579. |
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